论文标题

用于主动胶体运输的超材料

Metamaterials for Active Colloid Transport

论文作者

Yazdi, Shahrzad, Aragones, Juan L., Coulter, Jennifer, Alexander-Katz, Alfredo

论文摘要

在非平衡系统中的运输现象在生物学,工程和物理学中的无数应用中非常重要。复杂的环境,例如细胞质或多孔培养基,可能会严重影响此类系统的运输特性。特别是,最近的兴趣集中在这种环境如何影响主动系统的运动上,例如由方向驱动力推动的胶体和生物。然而,尽管合成系统和自然系统中旋转运动模式的无处不在,但具有非方向性(旋转)活性的主动物质运输尚未了解。在这里,我们报告了时空超材料系统的发现,这些系统能够基于两个参数来决定以精美的方式来决定旋转胶体的运输:时间的旋转调制频率和超材料的对称性。我们证明,用旋转对称性的晶格中自旋振幅的动态调节产生了非平衡的弹道传输带,使人联想到浮雕蓝o鱼系统中的弹性传输带。通过将这些时间调制与晶格中的其他对称性断裂耦合,我们显示了从4路到2向到单向运动的选择性控制。我们的结果为复杂(生物)系统中旋转物质运动的运动提供了关键的新见解。此外,我们的工作还可以用于设计具有新颖和独特的传输属性的系统,以便在例如无智能通道的微流体,微型机器人或胶体分离中进行应用。

Transport phenomena in out-of-equilibrium systems is immensely important in a myriad of applications in biology, engineering and physics. Complex environments, such as the cytoplasm or porous media, can substantially affect the transport properties of such systems. In particular, recent interest has focused on how such environments affect the motion of active systems, such as colloids and organisms propelled by directional driving forces. Nevertheless, the transport of active matter with non-directional (rotational) activity is yet to be understood, despite the ubiquity of rotating modes of motion in synthetic and natural systems. Here, we report on the discovery of spatiotemporal metamaterial systems that are able to dictate the transport of spinning colloids in exquisite ways based on solely two parameters: frequency of spin modulation in time and the symmetry of the metamaterial. We demonstrate that dynamic modulations of the amplitude of spin on a colloid in lattices with rotational symmetry give rise to non-equilibrium ballistic transport bands, reminiscent of those in Floquet-Bloch systems. By coupling these temporal modulations with additional symmetry breaking in the lattice, we show selective control from 4-way to 2-way to unidirectional motion. Our results provide critical new insights into the motion of spinning matter in complex (biological) systems. Furthermore, our work can also be used for designing systems with novel and unique transport properties for application in, for example, smart channel-less microfluidics, micro-robotics, or colloidal separations.

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