论文标题
通过群体感应的活动胶体悬浮液的相分离
A phase separation of active colloidal suspension via Quorum-sensing
论文作者
论文摘要
我们介绍了在两个维度上进行活性胶体悬浮液的布朗动力学模拟,其中胶体的自动螺旋速度受到局部密度的调节。详细研究了浓度依赖性运动在胶体及其动力学方面的作用。有趣的是,系统阶段以非常低的填充分数($φ\约0.125 $)分离,以较高的自行速度($ \ \ \ text {pe} $)分离,该速度与均匀阶段并存,并在过渡点以外的远程结晶顺序。从局部密度剖面,局部和全局池塘顺序参数量化了过渡点。我们已经表明,相图的特性在质量上类似于活性布朗粒子(ABP)模型。此外,我们的调查表明,密度依赖性的运动性放大了定向速度的慢速下降,这即使在低填充分数下也促进了相位分离。有效的扩散率显示了从二次上升到指数$ 3/2 $的幂律行为,并在相位分离的制度中带有$ \ text {pe} $。此外,我们已经表明,有效扩散在相位分离状态下随着填充分数的指数下降而降低,而单相方案的线性降低。
We present the Brownian dynamics simulation of active colloidal suspension in two dimensions, where the self-propulsion speed of a colloid is regulated according to the local density sensed by it. The role of concentration-dependent motility on the phase-separation of colloids and their dynamics is investigated in detail. Interestingly, the system phase separates at a very low packing fraction ($Φ\approx 0.125$) at higher self-propulsion speeds ($\text{Pe}$), which coexists with a homogeneous phase and attains long-range crystalline order beyond a transition point. The transition point is quantified here from the local density profiles, local and global-bond order parameters. We have shown that the phase diagram's characteristics are qualitatively akin to the active Brownian particle (ABP) model. Moreover, our investigation reveals that the density-dependent motility amplifies the slow-down of the directed speed, which facilitates phase-separation even at low packing fractions. The effective diffusivity shows a crossover from quadratic rise to a power-law behavior of exponent $3/2$ with $\text{Pe}$ in the phase-separated regime. Furthermore, we have shown that the effective diffusion decreases exponentially with packing fraction in the phase-separated regime while linear decrease in the single phase regime.