论文标题

单泡扩散生长期间超声增强的传质

Ultrasound-enhanced mass transfer during single-bubble diffusive growth

论文作者

Soto, Álvaro Moreno, Peñas, Pablo, Lajoinie, Guillaume, Lohse, Detlef, van der Meer, Devaraj

论文摘要

已知超声可以增强催化和微流体应用中的表面气泡的生长并去除,但是尚不清楚整流扩散和微流现象对传质的贡献。我们量化了超声对单个球形CO $ _2 $气泡在过饱和水中生长的泡沫的扩散生长的影响。时间依赖时间的气泡尺寸,形状,振荡振幅和微流场。我们表明并解释了超声如何在体积共振期间最多可以增强表面气泡的扩散生长。壁的接近性迫使气泡非球体振荡,从而在共振过程中产生剧烈的流,从而导致对流为主的生长。

Ultrasound is known to enhance surface bubble growth and removal in catalytic and microfluidic applications, yet the contributions of rectified diffusion and microstreaming phenomena towards mass transfer remain unclear. We quantify the effect of ultrasound on the diffusive growth of a single spherical CO$_2$ bubble growing on a substrate in supersaturated water. The time dependent bubble size, shape, oscillation amplitude and microstreaming flow field are resolved. We show and explain how ultrasound can enhance the diffusive growth of surface bubbles by up to two orders of magnitude during volumetric resonance. The proximity of the wall forces the bubble to oscillate non-spherically, thereby generating vigorous streaming during resonance that results in convection-dominated growth.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源