论文标题

通过单层MOS中的电场效应来控制激子多体状态$ _2 $

Controlling exciton many-body states by the electric-field effect in monolayer MoS$_2$

论文作者

Klein, Julian, Hötger, Alexander, Florian, Matthias, Steinhoff, Alexander, Delhomme, Alex, Taniguchi, Takashi, Watanabe, Kenji, Jahnke, Frank, Holleitner, Alexander W., Potemski, Marek, Faugeras, Clément, Finley, Jonathan J., Stier, Andreas V.

论文摘要

我们报告了高磁场的门控单层MOS $ _2 $的磁光谱,最高为28T,并获得有关中性和带电的激子的多体相互作用的新见解,并具有不同的旋转和山谷纹理的居民指控。对于低电子掺杂处的中性激子,我们观察到由于偶尔自旋相互作用而引起的非线性山谷Zeeman偏移,该旋转链接取决于局部载体浓度。随着费米能量在系统中的其他相关能量尺度上的主导地位,磁光响应取决于在$ k/k^{\ prime} $ valleys中的完全自旋极化的Landau水平的职业。这表现为多体状态。我们的实验表明,单层半导体中的激子只是一个接近电荷中性的单个粒子玻色子。我们发现,从电荷中立性中,它平稳地过渡到具有独特的自旋谷风味的极化状态,该味道由Landau水平量化的旋转和山谷质地定义。

We report magneto-optical spectroscopy of gated monolayer MoS$_2$ in high magnetic fields up to 28T and obtain new insights on the many-body interaction of neutral and charged excitons with the resident charges of distinct spin and valley texture. For neutral excitons at low electron doping, we observe a nonlinear valley Zeeman shift due to dipolar spin-interactions that depends sensitively on the local carrier concentration. As the Fermi energy increases to dominate over the other relevant energy scales in the system, the magneto-optical response depends on the occupation of the fully spin-polarized Landau levels in both $K/K^{\prime}$ valleys. This manifests itself in a many-body state. Our experiments demonstrate that the exciton in monolayer semiconductors is only a single particle boson close to charge neutrality. We find that away from charge neutrality it smoothly transitions into polaronic states with a distinct spin-valley flavour that is defined by the Landau level quantized spin and valley texture.

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