论文标题
磁化动力学的超快高谐波纳米镜检查
Ultrafast high-harmonic nanoscopy of magnetization dynamics
论文作者
论文摘要
光诱导的磁化变化,例如全光开关,天核成核和场地自旋转移,分别在时间和空间上展开至飞秒和纳米。泵探针光谱和衍射研究表明,时空动力学可能会严重影响非平衡磁力演化。然而,相关时间尺度上的直接真实空间磁成像仍然具有挑战性。在这里,我们展示了使用圆形极化高谐波辐射的超快高谐波纳米镜检查,用于对飞秒磁化动力学的真实空间成像。我们观察到飞秒激光激发后纳米级旋转质地的可逆和不可逆演变。具体而言,我们将磁性磁体域和局部旋转结构绘制在CO/PD多层的局部旋转结构,其亚波长空间分辨率降至16 nm,并以40 fs暂时分辨率的局部磁化动力学来追踪局部磁化动力学。我们的方法使磁光成像的最高时空分辨率迄今为止。在手性和线性二科运动中表达的各种显微镜自由度具有极高敏感性的超快成像,我们设想了广泛的应用,这些应用涵盖了磁性,相变和载体动力学。
Light-induced magnetization changes, such as all-optical switching, skyrmion nucleation, and intersite spin transfer, unfold on temporal and spatial scales down to femtoseconds and nanometers, respectively. Pump-probe spectroscopy and diffraction studies indicate that spatio-temporal dynamics may drastically affect the non-equilibrium magnetic evolution. Yet, direct real-space magnetic imaging on the relevant timescale has remained challenging. Here, we demonstrate ultrafast high-harmonic nanoscopy employing circularly polarized high-harmonic radiation for real-space imaging of femtosecond magnetization dynamics. We observe the reversible and irreversible evolution of nanoscale spin textures following femtosecond laser excitation. Specifically, we map quenched magnetic domains and localized spin structures in Co/Pd multilayers with a sub-wavelength spatial resolution down to 16 nm, and strobosocopically trace the local magnetization dynamics with 40 fs temporal resolution. Our approach enables the highest spatio-temporal resolution of magneto-optical imaging to date. Facilitating ultrafast imaging with an extreme sensitivity to various microscopic degrees of freedom expressed in chiral and linear dichroism, we envisage a wide range of applications spanning magnetism, phase transitions, and carrier dynamics.