论文标题

设计器蜂窝状晶格中的分子偶极子

Molecular dipoles in designer honeycomb lattices

论文作者

Boudjada, Nazim, Buessen, Finn Lasse, Paramekanti, Arun

论文摘要

表面科学的光学晶格和发展中的超速原子的最新进展允许创建人工晶格以及对多体相互作用的控制。这样的系统提供了新的设置来研究以互动驱动的不稳定性和非平凡的拓扑结构。在本文中,我们探索了二维三角晶格上的分子电偶极子之间的相互作用,并在双装饰的蜂窝晶状体上跳跃,该蜂窝晶状体在主持迪拉克和平坦的乐队状态。我们表明,短距离偶极 - 偶极相互作用会导致订购到各种条纹和涡流晶体基态。我们使用模拟退火和蒙特卡洛方法研究了这些有序状态及其热转变作为相互作用范围的函数。对于零波动矢量逆齿端阶的特殊情况,结合偶极子电子相互作用并集成电子会导致偶极顺序的六状态时钟模型。最后,我们讨论了各种偶极顺序对电子带结构和状态局部隧道密度的影响。我们的工作可能与排列在Cu(111)表面上的“分子石墨烯”的研究有关,这些分子已使用扫描隧道光谱进行了探索,以及在光学晶格中的Ultracold Molecule-Fermion混合物。

Recent advances in ultracold atoms in optical lattices and developments in surface science have allowed for the creation of artificial lattices as well as the control of many-body interactions. Such systems provide new settings to investigate interaction-driven instabilities and non-trivial topology. In this paper, we explore the interplay between molecular electric dipoles on a two-dimensional triangular lattice with fermions hopping on the dual decorated honeycomb lattice which hosts Dirac and flat band states. We show that short-range dipole-dipole interaction can lead to ordering into various stripe and vortex crystal ground states. We study these ordered states and their thermal transitions as a function of the interaction range using simulated annealing and Monte Carlo methods. For the special case of zero wave vector ferrodipolar order, incorporating dipole-electron interactions and integrating out the electrons leads to a six-state clock model for the dipole ordering. Finally, we discuss the impact of the various dipole orders on the electronic band structure and the local tunneling density of states. Our work may be relevant to studies of "molecular graphene" -- CO molecules arranged on the Cu(111) surface -- which have been explored using scanning tunneling spectroscopy, as well as ultracold molecule-fermion mixtures in optical lattices.

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