论文标题
基于模型的定量方法来预测合金辐射引起的肿胀
Model-based quantitative methods to predict irradiation-induced swelling in alloys
论文作者
论文摘要
基于现有的低剂量实验或具有高剂量速率能量颗粒的辐射数据,在高剂量中子辐射下预测核反应堆结构材料的体积肿胀一直是安全评估和快速筛查核能系统中耐辐射的耐药物质的长期挑战。在这里,我们构建了一个额外的缺陷吸收模型,描述了通过考虑辐射过程中固有的其他缺陷下沉来描述辐射引起的肿胀作用,重型离子和中子产生的肿胀效应。基于此模型,我们建立了定量方法,以预测低剂量行为中的高剂量肿胀,并在剂量速率差异数量级时获得不同能量颗粒的等效辐射剂量。此外,我们提出了一个通用参数,以表征各种合金的肿胀电阻,并在不同的辐射条件下预测它们的辐射公差。这项工作提供了用于评估辐照诱导的结构材料肿胀作用的定量预测方法,这对于晚期核反应堆的安全和材料开发至关重要。
Predicting volume swelling of structural materials in nuclear reactors under high-dose neutron irradiations based on existing low-dose experiments or irradiation data with high-dose-rate energetic particles has been a long-standing challenge for safety evaluation and rapidly screening irradiation-resistant materials in nuclear energy systems. Here, we build an Additional Defect Absorption Model that describes the irradiation-induced swelling effects produced by energetic electrons, heavy-ions, and neutrons by considering additional defect sinks inherent in the irradiation process. Based on this model, we establish quantitative methods to predict high-dose swelling from low-dose behavior and obtain the equivalent irradiation dose for different energetic particles when the dose rates differ by several orders of magnitude. Furthermore, we propose a universal parameter to characterize the swelling resistance of various alloys and predict their radiation tolerances under different radiation conditions. This work provides quantitative prediction methods for evaluating irradiation-induced swelling effects of structural materials, which is critical to the safety and material development for advanced nuclear reactors.