论文标题
具有光循环中心的芳族化合物的功能化化合物
Functionalizing Aromatic Compounds with Optical Cycling Centers
论文作者
论文摘要
分子设计原理提供了指南，以增强具有较小原子的分子以实现所需的特性或功能。我们证明这些概念可用于创建一个可以连接到许多芳族配体的光学循环中心，从而可以从所得分子中散射许多光子而不改变分子振动状态。我们提供进一步的设计原则，以表明扩大这项工作的能力。这代表了朝着量子官能团迈出的重要步骤，量子官能团可以用作通用量子部分，可以连接到各种分子结构和表面。
Molecular design principles provide guidelines for augmenting a molecule with a smaller group of atoms to realize a desired property or function. We demonstrate that these concepts can be used to create an optical cycling center that can be attached to a number of aromatic ligands, allowing the scattering of many photons from the resulting molecules without changing the molecular vibrational states. We provide further design principles that indicate the ability to expand this work. This represents a significant step towards a quantum functional group, which may serve as a generic qubit moiety that can be attached to a wide range of molecular structures and surfaces.
