论文标题

在由超快自旋相互作用触发的抗铁磁绝缘子中发射相干THZ

Emission of coherent THz magnons in an antiferromagnetic insulator triggered by ultrafast spin-phonon interactions

论文作者

Rongione, E., Gueckstock, O., Mattern, M., Gomonay, O., Meer, H., Schmitt, C., Ramos, R., Saitoh, E., Sinova, J., Jaffrès, H., Mičica, M., Mangeney, J., Goennenwein, S. T. B., Geprägs, S., Kampfrath, T., Kläui, M., Bargheer, M., Seifert, T. S., Dhillon, S., Lebrun, R.

论文摘要

由于其超快自旋动力学,已经提出了抗铁磁材料作为新型窄带THZ Spintronic设备。但是,操纵其旋转动态仍然是一个关键的挑战,这是通过旋转轨道扭矩或直接的光激发来实现的关键挑战。在这里,我们在Nio/Pt的低阻尼薄膜中以1 Thz的形式展示了宽带THz(不一致)磁子(不一致)的磁子和窄带(相干)磁子的组合产生。我们在实验和建模中证明了NiO中磁化动力学的两个激发过程,一种非谐振瞬时光学自旋扭矩以及由超快PT激发引起的应变波诱导的THZ扭矩。这两种现象都通过相邻重金属层中的反旋转大厅效应发出THZ信号。我们分别揭示了两个激发过程的特征时间尺度,分别<50 fs和> 300 fs,从而开放了基于抗磁磁材料的快速光旋转设备开发的新途径。

Antiferromagnetic materials have been proposed as new types of narrowband THz spintronic devices owing to their ultrafast spin dynamics. Manipulating coherently their spin dynamics, however, remains a key challenge that is envisioned to be accomplished by spin-orbit torques or direct optical excitations. Here, we demonstrate the combined generation of broadband THz (incoherent) magnons and narrowband (coherent) magnons at 1 THz in low damping thin films of NiO/Pt. We evidence, experimentally and through modelling, two excitation processes of magnetization dynamics in NiO, an off-resonant instantaneous optical spin torque and a strain-wave-induced THz torque induced by ultrafast Pt excitation. Both phenomena lead to the emission of a THz signal through the inverse spin Hall effect in the adjacent heavy metal layer. We unravel the characteristic timescales of the two excitation processes found to be < 50 fs and > 300 fs, respectively, and thus open new routes towards the development of fast opto-spintronic devices based on antiferromagnetic materials.

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