论文标题

软材料中的单文件动态

Single file dynamics in soft materials

论文作者

Taloni, Alessandro, Flomenbom, Ophir, Castaneda-Priego, Ramon, Marchesoni, Fabio

论文摘要

术语单文件(SF)动力学是指颗粒组装通过通道的运动,其横截面与颗粒直径相当。然后,单文件扩散(SFD)是标记粒子在\ emph {单文件}中的扩散,即在不允许粒子传递的条件下。 SFD在自然界中说明了各种各样的过程,包括胶体在合成和天然形的通道中的扩散,沿分子链的生物电动机,蛋白质中的电子和液态氦气,通过膜,仅提及一些例子。尽管在过去的十年中,SF动力学的经典概念已被推广,以通过更真实的建模,包括颗粒性能,文件几何形状,粒子粒子和通道粒子相互作用,从而铺平了在bio-NananodeDectient的技术中,铺平了铺平的方法。然后,我们对SF动力学理论和随之而来的实验实现的最新进展进行了全面综述。

The term single file (SF) dynamics refers to the motion of an assembly of particles through a channel with cross-section comparable to the particles' diameter. Single file diffusion (SFD) is then the diffusion of a tagged particle in a \emph{single file}, i.e., under the condition that particle passing is not allowed. SFD accounts for a large variety of processes in nature, including diffusion of colloids in synthetic and natural-shaped channels, biological motors along molecular chains, electrons in proteins and liquid helium, ions through membrane, just to mention a few examples. Albeit introduced in '65, over the last decade the classical notion of SF dynamics has been generalized to account through a more realistic modeling of, among others, particles properties, file geometry, particle-particle and channel-particles interactions, thus paving the way to remarkable applications in, for example, the technology of bio-integrated nanodevices. We then provide a comprehensive review of the recent advances in the theory of SF dynamics and the ensuing experimental realisations.

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