论文标题

表面粗糙度噪声分析和全面噪声对钻石中NV中心深度相干时间的综合噪声影响

Surface roughness noise analysis and comprehensive noise effects on depth-dependent coherence time of NV centers in diamond

论文作者

Chrostoski, Philip, Kehayias, Pauli, Santamore, D. H.

论文摘要

噪声是钻石中氮呈(NV)中心的有害问题,导致线扩大并减少了相干时间(T2)。在我们先前的电场和磁场噪声工作之后,我们研究了由钻石表面粗糙度引起的噪声,这是电荷密度波动和不相互分光子散射的来源。我们发现,在整个NV动力学脱钩频率范围内,不同的表面电荷密度噪声源很普遍,而光子散射噪声几乎可以忽略不计。接下来,我们将各种噪声源的结果结合在一起,以对T2进行全面的分析,以及它如何随NV深度变化。在给定的NV深度低于氢或氟终止的表面下,我们发现这些磁核会减少NV相干时间,其次是表面电场噪声源。与电荷密度,电偶极子和表面杂质噪声相比,光子散射和大量磁场噪声对T2的效果较弱。但是,随着氧表面终止,表面电场噪声与表面磁场噪声相当。我们计算出的T2,Hahn(几微秒至十微秒)的值与其他地方报道的实验值非常吻合。最后,我们计算了外部核自旋的NV AC磁力测定法的预期信号噪声比(SNR)。在我们的简化评估中,在某些深度依赖性参数(例如NV转换效率)保持恒定时,我们发现较浅的NV层应产生最佳的SNR,这与实验发现一致。

Noise is a detrimental issue for nitrogen-vacancy (NV) centers in diamond, causing line broadening and decreasing the coherence time (T2). Following our previous electric and magnetic field noise work, we investigate noise caused by the diamond surface roughness, which is a source for charge density fluctuations and incoherent photon scattering. We find that the varying surface charge density noise source is prevalent throughout the entire NV dynamical decoupling frequency range, while the photon scattering noise is almost negligible. Next, we combine the results from various noise sources to perform comprehensive analyses on T2 and how it varies with NV depth. At a given NV depth of 5 nm below a hydrogen- or fluorine-terminated surface, we find that these magnetic nuclei reduce the NV coherence time the most, followed by the surface electric field noise sources. The photon scattering and bulk magnetic field noise effects on T2 are weak compared to the varying charge density, electric dipole, and surface impurity noise. However, with oxygen surface termination, the surface electric field noise becomes comparable to the surface magnetic field noise. Our calculated values of T2,Hahn (few microseconds to ten microseconds) are in good agreement with the experimental values reported elsewhere. Finally, we calculate an anticipated signal-to-noise ratio (SNR) for NV AC magnetometry of external nuclear spins. In our simplified assessment, where some depth-dependent parameters (e.g. NV conversion efficiency) are held constant, we find that shallower NV layers should yield the best SNR, which is consistent with experimental findings.

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