学术文献库

Modern electron microscopy and spectroscopy is a key technology for studying the structure and composition of quantum and biological materials in fundamental and applied sciences. High-resolution spectroscopic techniques and aberration-corrected microscopes are often limited by the relatively large energy distribution of currently available beam sources. This can be improved by a monochromator, with the significant drawback of losing most of the beam current. Here, we study the field emission properties of a monocrystalline niobium tip electron field emitter at 5.2 K, well below the superconducting transition temperature. The emitter fabrication process can generate two tip configurations, with or without a nano-protrusion at the apex, strongly influencing the field-emission energy distribution. The geometry without the nano-protrusion has a high beam current, long-term stability, and an energy width of around 100 meV. The beam current can be increased by two orders of magnitude by xenon gas adsorption. We also studied the emitter performance up to 82 K and demonstrated the beam's energy width can be below 40 meV even at liquid nitrogen cooling temperatures when an apex nano-protrusion is present. Furthermore, the spatial and temporal electron-electron correlations of the field emission are studied at normal and superconducting temperatures and the influence of Nottingham heating is discussed. This new monochromatic source will allow unprecedented accuracy and resolution in electron microscopy, spectroscopy, and high-coherence quantum applications.