论文标题
元素稀释效果对非kramers系统的四极临界效应y $ _ $ _ {1-x} $ pr $ _x $ ir $ _2 $ _2 $ zn $ _ {20} $
Elemental Dilution Effect on the Elastic Response due to a Quadrupolar Kondo Effect of the Non-Kramers System Y$_{1-x}$Pr$_x$Ir$_2$Zn$_{20}$
论文作者
论文摘要
我们测量了非kramers System $ \ rm \ rm \ rm \ rm {y_ {0.63} pr_ {0.63} pr_ {0.37} ir_ {2} ir_ {2} zn_ {2} zn_ {20} $(pr y yll of Mull of Mull of Enctall ostect)单位四极近极效应通过增加PR浓度来改变。 The Curie-like softening of $\left(C_{11}-C_{12}\right)/2$ between 1 and 5 K of the present Pr-37% system can be reproduced by a multipolar susceptibility calculation based on the non-Kramers $Γ_3$ doublet crystalline-electric-field ground state.此外,在低于0.15 K的冷却时,在$ \ left(c_ {11} -c_ {12} \ right)/2 $中观察到与$ \ sqrt {t} $成比例的温度依赖性。与PR-3.4%系统不同的是,这种行为对应于四极近相结构“晶格”模型的理论预测,该模型与PR-3.4%系统不同,该系统显示了基于“单位点”四极性近关系理论的对数温度依赖性。此外,我们讨论了通过在PR-37%系统中的非kramer Doublet的低能声子与非kramer double的电二核之间的耦合形成振动状态的可能性,因为我们发现在0.15至1 k之间的温度区域中有低能的超声分散体。
We measured the elastic constants $\left(C_{11}-C_{12}\right)/2$ and $C_{44}$ of the non-Kramers system $\rm{Y_{0.63}Pr_{0.37}Ir_{2}Zn_{20}}$ (Pr-37% system) by means of ultrasound to check how the single-site quadrupolar Kondo effect is modified by increasing the Pr concentration. The Curie-like softening of $\left(C_{11}-C_{12}\right)/2$ between 1 and 5 K of the present Pr-37% system can be reproduced by a multipolar susceptibility calculation based on the non-Kramers $Γ_3$ doublet crystalline-electric-field ground state. Further, on cooling below 0.15 K, a temperature dependence proportional to $\sqrt{T}$ was observed in $\left(C_{11}-C_{12}\right)/2$. This behavior rather corresponds to the theoretical prediction of the quadrupolar Kondo "lattice" model, unlike that of the Pr-3.4% system, which shows a logarithmic temperature dependence based on the "single-site" quadrupolar Kondo theory. In addition, we discuss the possibility to form a vibronic state by the coupling between the low-energy phonons and the electric quadrupoles of the non-Kramers doublet in the Pr-37% system, since we found a low-energy ultrasonic dispersion in the temperature region between 0.15 and 1 K.